Document Type

Article

Original Publication Date

2002

Journal/Book/Conference Title

Journal of Applied Physics

Volume

91

Issue

10

DOI of Original Publication

10.1063/1.1450786

Comments

Originally published at http://dx.doi.org/10.1063/1.1450786

Date of Submission

October 2015

Abstract

We have performed density-functional-based electronic structure calculations on a single Fe8 molecular nanomagnet. Our calculated total moments and local moments are in excellent agreement with experiment. By including spin–orbit coupling we determine the easy, medium, and hard axes and find the ordering of the principle axes also agrees with experiment. From our calculated anisotropy Hamiltonian, we calculate the oscillations in the tunnel splittings and compare to the experimental results.

Rights

Pederson, M. R., Kortus, J., Khanna, S. N. Electronic-structure-based investigation of magnetism in the Fe8 molecular magnet. Copyright © 2002 AIP Publishing LLC.

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VCU Physics Publications

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