Document Type

Article

Original Publication Date

1996

Journal/Book/Conference Title

Journal of Chemical Physics

Volume

105

Issue

24

DOI of Original Publication

10.1063/1.472901

Comments

Originally published at http://dx.doi.org/10.1063/1.472901

Date of Submission

October 2015

Abstract

The equilibrium geometries, binding energies, and electronic structure of neutral FeC n (n≤3) clusters have been calculated self‐consistently using ab initio molecular orbital theory. The exchange and correlation contributions to the total energy were computed using both the density functional method (with and without nonlocal correction) as well as the Hartree–Fock–Möller–Plesset theory. All levels of theory predict the equilibrium geometries to be cyclic. The binding energies, bond lengths, and the Mulliken charges obtained from both methods of calculations are also in agreement. The results are compared with recent mobility and photoelectron spectroscopy experiments.

Rights

Nash, B. K., Rao, B. K., & Jena, P. Equilibrium structure and bonding of small iron-carbon clusters. The Journal of Chemical Physics, 105, 11020 (1996). Copyright © 1996 American Institute of Physics.

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