Document Type

Article

Original Publication Date

1997

Journal/Book/Conference Title

Journal of Chemical Physics

Volume

107

Issue

1

DOI of Original Publication

10.1063/1.474360

Comments

Originally published at http://dx.doi.org/10.1063/1.474360

Date of Submission

October 2015

Abstract

Ab initio molecular orbital theory based on both density functional formalism and quantum chemical methods has been used to calculate the equilibrium geometries, binding energies, ionization potentials, fragmentation patterns, and electronic structures of neutral and charged boron clusters containing up to six atoms. Calculations have also been performed on restricted geometries for BnX (n=1,5,12; X=Be, B, C) and B20 clusters to see if clusters can be designed so as to increase their stability. Energetics of doubly chargedB++n clusters have also been studied to find the critical size for Coulomb explosion. The results are compared with existing experimental and theoretical data.

Rights

Niu, J., Rao, B. K., & Jena, P. Atomic and electronic structures of neutral and charged boron and boron-rich clusters. The Journal of Chemical Physics, 107, 132 (1997). Copyright © 1997 American Institute of Physics.

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