Document Type

Article

Original Publication Date

2019

Journal/Book/Conference Title

Polymers

Volume

11

Issue

9:1406

First Page

1

Last Page

11

DOI

10.3390/polym11091406

Comments

Originally published at https://doi.org/10.3390/polym11091406.

Funded in part by the VCU Libraries Open Access Publishing Fund.

Date of Submission

December 2019

Abstract

Flash NanoPrecipitation (FNP) is a rapid method for encapsulating hydrophobic materials in polymer nanoparticles with high loading capacity. Encapsulating biologics such as proteins remains a challenge due to their low hydrophobicity (logP < 6) and current methods require multiple processing steps. In this work, we report rapid, single-step protein encapsulation via FNP using bovine serum albumin (BSA) as a model protein. Nanoparticle formation involves complexation and precipitation of protein with tannic acid and stabilization with a cationic polyelectrolyte. Nanoparticle self-assembly is driven by hydrogen bonding and electrostatic interactions. Using this approach, high encapsulation efficiency (up to ~80%) of protein can be achieved. The resulting nanoparticles are stable at physiological pH and ionic strength. Overall, FNP is a rapid, efficient platform for encapsulating proteins for various applications.

Rights

© 2019 by the authors. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).

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VCU Chemical and Life Science Engineering Publications

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Engineering Commons

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