Defense Date

2024

Document Type

Dissertation

Degree Name

Doctor of Philosophy

Department

Nanoscience and Nanotechnology

First Advisor

Joseph Reiner

Second Advisor

Jason Reed

Third Advisor

Indika Arachchige

Fourth Advisor

Richard Inho Joh

Abstract

The early detection of disease is paramount for ensuring survival and quality of life for patients. Ovarian cancer, currently one of the leading causes of death in women, generally still lacks early screening methodologies which can effectively detect cases in the early stages. The emergence of protein and peptide biomarkers in biological fluids appears promising to this end, specifically Leucine Rich Glycoprotein(LRG-1) which is found at high elevated concentrations in the urine of ovarian cancer patients.

In this research we have shown that nanoparticle assisted nanopore detection can serve as an effective label-free technique for detecting and discriminating peptide fragments generated from the digestion of the LRG-1 protein in biological fluids. This technique takes advantage of cysteine selective detection in order to target peptides and reject the complex background that exists in urine samples. This method shows great promise for development into a low-cost point of care assay for the detection of peptide biomarkers for the early screening of ovarian cancer.

Rights

© The Author

Is Part Of

VCU University Archives

Is Part Of

VCU Theses and Dissertations

Date of Submission

5-7-2024

Available for download on Monday, May 07, 2029

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