Author ORCID Identifier

https://orcid.org/0009-0009-0553-6254

Defense Date

2026

Document Type

Thesis

Degree Name

Master of Science

Department

Biology

First Advisor

Jason Newton

Abstract

The correlation between incidences of neurodegenerative disease and exposure to the non-proteinogenic amino acid β-N-methylamino-L-alanine (BMAA), first observed in Guam in the 1950s, prompted an investigation of its neurotoxic effects. Further research linked BMAA exposure to neurodegenerative diseases characterized as amyotrophic lateral sclerosis- Parkinsonism-dementia complex (ALS/PDC); now mainly attributed to sporadic ALS (sALS). The mechanism of BMAA’s toxicity is not currently understood, with previous research focusing on its misincorporation during protein synthesis, this mechanism remains difficult to validate in vivo. Therefore, this thesis investigates an alternative mechanism in which BMAA disrupts de novo sphingolipid biosynthesis by substituting itself for L-serine and giving rise to atypical sphingolipid species. Using multiple model systems, this research shows that BMAA perturbs sphingolipid metabolism, induces developmental malformations, impairs locomotor behavior and growth, and contributes to central nervous system deficits at the motor axon level. This study further demonstrates that L-serine mitigates BMAA-associated developmental abnormalities and is neuroprotective of motor axon reduction in zebrafish embryos. In addition, LC-ESI-MS/MS analysis identifies novel sphingolipid species, 1-methylamino-dihydroceramides, consistent with the lipid incorporation mechanism of BMAA. Together, these findings support a mechanism of BMAA neurotoxicity mediated by incorporation in sphingolipid synthesis and provide evidence for L-serine as a protective modifier of these effects.

Rights

© The Author

Is Part Of

VCU University Archives

Is Part Of

VCU Theses and Dissertations

Date of Submission

5-8-2026

Available for download on Sunday, May 07, 2028

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