Document Type

Article

Original Publication Date

2008

Journal/Book/Conference Title

The Journal of Chemical Physics

Volume

129

Issue

7

DOI of Original Publication

10.1063/1.2968609

Comments

Originally published at http://dx.doi.org/10.1063/1.2968609

Date of Submission

October 2015

Abstract

Fem(coronene)n (m=1,2, n=1,2) cluster anions were generated by a laser vaporization source and studied by anion photoelectron spectroscopy. Density functional theory was used to calculate the structures and the spin multiplicities of those clusters as well as the electron affinities and photodetachment transitions. The calculated magnetic moments of Fe1(coronene)1 and Fe2(coronene)1 clusters suggest that coronene could be a suitable template on which to deposit small iron clusters and that these in turn might form the basis of an iron cluster-based magnetic material. Fe1(coronene)2 and Fe2(coronene)2 cluster anions and their corresponding neutrals prefer the sandwich-type structures, and the ground state structures of these clusters are all staggered sandwiches.

Rights

Li, X., Eustis, S., Bowen, K. H., et al. Photoelectron spectroscopic and theoretical studies of Fem−(coronene)n (m=1,2, n=1,2) complexes. The Journal of Chemical Physics 129, 074313 (2008). Copyright © 2008 AIP Publishing LLC.

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