Author ORCID Identifier

https://orcid.org/0009-0001-1953-9415

Defense Date

2024

Document Type

Thesis

Degree Name

Master of Science

Department

Chemical and Life Science Engineering

First Advisor

Dr. James K. Ferri

Abstract

Continuous pharmaceutical manufacturing involves converting chemical reactants into active pharmaceutical ingredients via chemical transformation in interconnected vessels and flow reactors. These techniques and the associated advantages can be an essential strategy for reducing manufacturing costs and addressing shortages of lifesaving drugs. Due to purity requirements in the pharmaceutical industry, developing robust and reliable purification techniques is a significant area of interest regarding continuous manufacturing. This work discusses general drug salt purification steps within continuous manufacturing, including salt formation, crystallization, and an area of research that shows potential for use as a process intensification tool for continuous separations: tangential flow filtration (TFF). TFF is established in the pharmaceutical industry, but limited research exists for continuous separation of small molecule drug slurries. Experiments and design considerations for purification using TFF and distillation are explored as a basis for developing reusable pattern-based archetypes for separations processes. The use of commercially available, micro-filtration membranes as a multi-purpose unit operation for continuous drug salt processing and the design of a tailored distillation column are discussed within the context of a continuous albuterol sulfate manufacturing system. Results highlight solid removal, product concentration, and product washing applications of TFF leading to reduced filter-dryer cycle time and increased product throughput up to 30%. Distillation design was conducted utilizing experimentally determined equilibrium data and ASPEN+ software as a process development tool. The case-studies presented showcase TFF and distillation technologies as a continuous manufacturing tool to facilitate process intensification steps and continuously process API slurries in the pharmaceutical industry.

Rights

© The Author

Is Part Of

VCU University Archives

Is Part Of

VCU Theses and Dissertations

Date of Submission

5-9-2024

Available for download on Tuesday, May 08, 2029

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